图文目录｜GEE Volume 7, Issue 5 正式出版
Green Energy & Environment
Volume 7
Issue 5
Green Energy & Environment 2022年第七卷第五期已正式出版。本期共收录文章23篇，其中research highlight 1篇，review article 2篇，research paper 20篇。欢迎大家阅读、下载和投稿！
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封面文章
中山大学严凯教授课题组研究论文——Green fabrication of nickel-iron layered double hydroxides nanosheets efficient for the enhanced capacitive performance封底文章
厦门大学生物质燃料与化学品团队综述论文——Catalyst design strategy toward the efficient heterogeneously-catalyzed selective oxidation of 5-hydroxymethylfurfural厦门大学生物质燃料与化学品团队对已建立的通过热催化氧化HMF的异相催化剂设计策略进行了综述，并分析了该领域当前面临的挑战和未来发展方向。该论文第一作者为刘淮博士，现工作于昆明理工大学，通讯作者为厦门大学唐兴副教授。
该作品以绿色森林和草地为背景，通过一股“风”将5-羟甲基糠醛氧化为高附加值的化学品，并最终得到“塑料瓶”。绿色森林和草地的背景表示原料来源于生物质，而带有不同催化剂的“风”象征着催化反应过程，而最终得到的“塑料瓶”表示可以通过这种方式生产可再生的化学品及材料。
图文目录
Research highlight
Exclusive CO2-to-formate conversion over single-atom alloyed Cu-based catalysts
Junjun Li, Zhicheng Zhang*, Wenping Hu
https://doi.org/10.1016/j.gee.2021.11.004
Citation: J. Li, Z. Zhang, W. Hu, Green Energy Environ. 7 (2022) 855.
Review articles
Understanding of the electrochemical behaviors of aqueous zinc–manganese batteries: Reaction processes and failure mechanisms
Xinyu Luo, Wenchao Peng, Yang Li, Fengbao Zhang, Xiaobin Fan*https://doi.org/10.1016/j.gee.2021.08.006
Citation: X. Luo, W. Peng, Y. Li, F. Zhang, X. Fan, Green Energy Environ. 7 (2022) 858-899.
天津大学范晓彬教授团队GEE综述：对于水系锌−锰电池的电化学行为的理解——反应过程和失效机制
Catalyst design strategy toward the efficient heterogeneously-catalyzed selective oxidation of 5-hydroxymethylfurfural
Huai Liu, Xing Tang*, Xianhai Zeng, Yong Sun, Xixian Ke, Tianyuan Li, Jiaren Zhang, Lu Lin
To improve the catalytic performance of the catalysts for the oxidation of 5-(hydroxymethyl)furfural (HMF), various catalyst design strategies have been developed to modify the geometric as well as the electronic configurations of the active centers, which have been systematically summarized in this review.
https://doi.org/10.1016/j.gee.2021.10.004
Citation: H. Liu, X. Tang, X. Zeng, Y. Sun, X. Ke, T. Li, J. Zhang, L. Lin, Green Energy Environ. 7 (2022) 900-932.
厦门大学生物质燃料与化学品团队GEE：催化氧化5-羟甲基糠醛的异相催化剂设计策略
Research papers
Pd nanocluster-decorated CoFe composite supported on nitrogen carbon nanotubes as a high-performance trifunctional electrocatalyst
Revanasiddappa Manjunatha, Li Dong, Zibo Zhai, Jianyi Wang, Qianru Fu, Wei Yan*, Jiujun Zhang*
Pd nanocluster-decorated CoFe double-layered composite supported on nitrogen carbon nanotubes as a high-performance trifunctional electrocatalyst for water electrolysis and flexible Zinc-air battery applications.
https://doi.org/10.1016/j.gee.2020.12.005
Citation: R. Manjunatha, L. Dong, Z. Zhai, J. Wang, Q. Fu, W. Yan, J. Zhang, Green Energy Environ. 7 (2022) 933-947.
High retention volume covalent organic polymer for xenon capture: Dynamic separation of Xe and Kr
Qian Wang1, Zhu Meng1, Juntao Li, Shuming Peng*, Zhonghua Xiang*
A new covalent organic polymer COP-14 is developed for Xe/Kr separation. Suitable pore size and structure make it successfully separates low concentration Xe (350 ppm) and Kr (35 ppm) in dynamic breakthrough experiments.
https://doi.org/10.1016/j.gee.2020.12.010
Citation: Q. Wang, Z. Meng, J. Li, S. Peng, Z. Xiang, Green Energy Environ. 7 (2022) 948-956.
Na-MnOx catalyzed aerobic oxidative cleavage of biomass-derived 1,2-diols to synthesis medium-chain furanic chemicals
Qing-Shan Kong, Xing-Long Li, Hong-Bo Shen, Hua-Jian Xu*, Yao Fu*
A strategy based on furanic platform chemicals was developed to synthesize a variety of high value-added furan-based compounds (diacids and esters, diols, hydroxy acids, acrylics), which simultaneously utilizes Na-MnOx catalyst and practical catalytic methods.
https://doi.org/10.1016/j.gee.2020.12.007
Citation: Q.-S. Kong, X.-L. Li, H.-B. Shen, H.-J. Xu, Y. Fu, Green Energy Environ. 7 (2022) 957-964.
Magnetically enhancing diffusion for dendrite-free and long-term stable lithium metal anodes
Yongxiu Chen, Xiangyu Dou, Kai Wang, Yongsheng Han*
An introduction of external magnetic field vertical to the anode in lithium batteries leads to an enhanced even distribution of lithium ions at the surface, resulting in a dendrite-free lithium deposition.
https://doi.org/10.1016/j.gee.2020.12.014
Citation: Y. Chen, X. Dou, K. Wang, Y. Han, Green Energy Environ. 7 (2022) 965-974.
Scaled-up synthesis of defect-rich layered double hydroxide monolayers without organic species for efficient oxygen evolution reaction
Haoyuan Chi1, Jingwen Dong1, Tian Li1, Sha Bai, Ling Tan, Jikang Wang, Tianyang Shen, Guihao Liu, Lihong Liu, Luyi Sun, Yufei Zhao*, Yu-Fei Song*
Through the separate nucleation and aging steps by using colloid mill reactor, monolayer LDHs were synthesized on a large scale. The defects-rich monolayer LDHs obtained by this method showed efficient electrocatalytic activity for oxygen evolution reaction.
https://doi.org/10.1016/j.gee.2020.12.013
Citation: H. Chi, J. Dong, T. Li, S. Bai, L. Tan, J. Wang, T. Shen, G. Liu, L. Liu, L. Sun, Y. Zhao, Y.-F. Song, Green Energy Environ. 7 (2022) 975-982.
Efficient catalytic removal of COS and H2S over graphitized 2D micro-meso-macroporous carbons endowed with ample nitrogen sites synthesized via mechanochemical carbonization
Xun Kan1, Guanqing Zhang1, Yingying Luo, Fujian Liu*, Yong Zheng, Yihong Xiao, Yanning Cao, Chak-tong Au, Shijing Liang*, Lilong Jiang
Graphitized 2D micro-meso-macroporous carbons endowed with ultrahigh concentration of structural base nitrogen sites were synthesized by a one-step mechanochemical carbonization route. The samples act as high-efficient and stable catalysts for conversion of COS and H2S to elemental sulfur.
https://doi.org/10.1016/j.gee.2020.12.016
Citation: X. Kan, G. Zhang, Y. Luo, F. Liu, Y. Zheng, Y. Xiao, Y. Cao, C.-t. Au, S. Liang, L. Jiang, Green Energy Environ. 7 (2022) 983-995.
Synthesis and fluorescent properties of quinoxaline derived ionic liquids
Jiaqi Wu, Lei Zhang, Jinxing Long, Qiang Zeng, Biaolin Yin*, Xuehui Li*
Based on a two-step process including a dual Schiff's base formation and a [RhCp∗Cl2]2-catalyzed oxidative C–H activation/annulation, a series of novel fluorescent isoquinolino [2,1-a]quinoxalin-5-ium ionic liquids (ILs) were prepared, showing dual or triple emissions due to the local excited state, charge transfer state and excited state proton transfer state of cation.
https://doi.org/10.1016/j.gee.2020.12.018
Citation: J. Wu, L. Zhang, J. Long, Q. Zeng, B. Yin, X. Li, Green Energy Environ. 7 (2022) 996-1005.
Building of multifunctional and hierarchical HxMoO3/PNIPAM hydrogel for high-efficiency solar vapor generation
Shuai Cao1, Jingyun Jiang1, Qingyong Tian*, Cang Guo, Xuzhe Wang, Kun Dai, Qun Xu*
A novel multifunctional and hierarchically nanostructured HxMoO3/PNIPAM hydrogel with photothermal activity and activate water capacity was achieved via one-step polymerization. The HxMoO3-contained hydrogel solar evaporator device fabricated here possesses a competitive water evaporation rate of 1.65 kg m-2 h-1 with the energy efficiency of 85.87% under 1 kW m-2 irradiation.
https://doi.org/10.1016/j.gee.2020.12.012
Citation: S. Cao, J. Jiang, Q. Tian, C. Guo, X. Wang, K. Dai, Q. Xu, Green Energy Environ. 7 (2022) 1006-1013.
The influence of pore structures and Lewis acid sites on selective hydrogenolysis of guaiacol to benzene over Ru/TS-1
Yingying Xin, Zhaoxia Zheng, Zhicheng Luo*, Chengzhen Jiang, Shaofeng Gao, Zhihao Wang, Chen Zhao*
Pore structure properties of MFI coupled with abundant LAS (TS-1) as well as Ru NPs on the orifice of pores of TS-1 promotes the hydrogenolysis of lignin to aromatics, while BAS on Ru/MFI promotes the hydrogenation rates of aromatics.
https://doi.org/10.1016/j.gee.2020.12.024
Citation: Y. Xin, Z. Zheng, Z. Luo, C. Jiang, S. Gao, Z. Wang, C. Zhao, Green Energy Environ. 7 (2022) 1014-1023.
Engineering heterostructured Ni@Ni(OH)2 core-shell nanomaterials for synergistically enhanced water electrolysis
Jun-Wei Zhang1, Xian-Wei Lv1, Tie-Zhen Ren*, Zheng Wang, Teresa J. Bandosz, Zhong-Yong Yuan*https://doi.org/10.1016/j.gee.2020.12.009
Citation: J.-W. Zhang, X.-W. Lv, T.-Z. Ren, Z. Wang, T.J. Bandosz, Z.-Y. Yuan, Green Energy Environ. 7 (2022) 1024-1032.
Synthesis of ordered hierarchically mesoporous/microporous carbon materials via compressed CO2 for fructose-to-HMF transformation
Sen Luan, Wei Li*, Zanwu Guo, Wenxiu Li, Xiaojian Hou, Yi Song, Ran Wang, Qian Wang
A well-ordered hierarchically porous carbon (HPC) materiel was fabricated via dual soft-templating approach with compressed CO2. The as-prepared HPC sample as the catalysis carrier exhibited the excellent catalytic performance with high HMF yield and accelerated reaction rate in the fructose-to-HMF transformation.
https://doi.org/10.1016/j.gee.2021.01.005
Citation: S. Luan, W. Li, Z. Guo, W. Li, X. Hou, Y. Song, R. Wang, Q. Wang, Green Energy Environ. 7 (2022) 1033-1044.
Ga2OSe monolayer: A promising hydrogen evolution photocatalyst screened from two-dimensional gallium chalcogenides and the derived janus
Yu Cui, Mengyuan Li, Xiaoli Zhang, Sufan Wang, Yucheng Huang*https://doi.org/10.1016/j.gee.2021.01.002
Citation: Y. Cui, M. Li, X. Zhang, S. Wang, Y. Huang, Green Energy Environ. 7 (2022) 1045-1052.
Green fabrication of nickel-iron layered double hydroxides nanosheets efficient for the enhanced capacitive performance
Yuchen Wang, Zuo Chen, Man Zhang, Yaoyu Liu, Huixia Luo*, Kai Yan*https://doi.org/10.1016/j.gee.2021.01.019
Citation: Y. Wang, Z. Chen, M. Zhang, Y. Liu, H. Luo, K. Yan, Green Energy Environ. 7 (2022) 1053-1061.
Analyzing acetylene adsorption of metal–organic frameworks based on machine learning
Peisong Yang, Gang Lu*, Qingyuan Yang*, Lei Liu, Xin Lai, Duli Yu
The article uses machine learning methods to build an accurate prediction model of MOFs' adsorption capacity for C2H2. According to the classification model, effective design rules are extracted, which is of great significance to the selection and design of materials.
https://doi.org/10.1016/j.gee.2021.01.006
Citation: P. Yang, G. Lu, Q. Yang, L. Liu, X. Lai, D. Yu, Green Energy Environ. 7 (2022) 1062-1070.
Carbonized waste milk powders as cathodes for stable lithium–sulfur batteries with ultra-large capacity and high initial coulombic efficiency
Rabia Khatoon, Sanam Attique, Rumin Liu, Sajid Rauf, Nasir Ali, Luhong Zhang, Yu-Jia Zeng*, Yichuan Guo, Yusuf Valentino Kaneti*, Jongbeom Na, Haichao Tang, Hongwen Chen, Yang Tian, Jianguo Lu*
A trash to treasure approach to utilize waste milk powders as cathode in Li–S batteries. Cathode comprises of CMP/S (1:2) exhibited best electrochemical performance compared to CMP/S (1:1) and CMP/S (1:3).
https://doi.org/10.1016/j.gee.2021.01.007
Citation: R. Khatoon, S. Attique, R. Liu, S. Rauf, N. Ali, L. Zhang, Y.-J. Zeng, Y. Guo, Y.V. Kaneti, J. Na, H. Tang, H. Chen, Y. Tian, J. Lu, Green Energy Environ. 7 (2022) 1070-1083.
Vitamin B9 derived nitrogen-doped graphene for metal-free aerobic oxidation of biomass-derived chemicals
Duan-Jian Tao*, Xin Zhao, Yanxin Wang, Xixi Liu, Hong-Ping Li, Zhang-Min Li, Yan Zhou, Ziliang Yuan, Zehui Zhang*
A superior carbocatalyst ultrahigh N-doped graphene (NG) was prepared by a novel self-sacrificial templating method of one-step annealing vitamin B9. Systematic characterizations and quantum-chemical calculations further manifested that high contents of graphitic N and pyridinic N species in VB9-NG-800 promoted the generation of •O2− active species from molecular oxygen effortlessly, resulting in excellent catalytic performance for aerobic oxidation.
https://doi.org/10.1016/j.gee.2021.01.008
Citation: D.-J. Tao, X. Zhao, Y. Wang, X. Liu, H.-P. Li, Z.-M. Li, Y. Zhou, Z. Yuan, Z. Zhang, Green Energy Environ. 7 (2022) 1084-1092.
A succinct enhanced luminescence strategy for fluorescent ionic liquids and the application for detecting CO2
Siying Che, Jiachen Guo, Lu Gan, Qiaoxin Xiao, Haoran Li, Yuanbin She, Congmin Wang*
We reported a succinct enhanced luminescence strategy to reduce single-triplet energy split using the tunability of ionic liquids; thus up to 15 fold enhancements were achieved. This fluorescence ionic liquid has the advantages of a simple synthesis, convenient regulation and a remarkable effect, which has a good potential for detecting gas such as CO2.
https://doi.org/10.1016/j.gee.2021.01.010
Citation: S. Che, J. Guo, L. Gan, Q. Xiao, H. Li, Y. She, C. Wang, Green Energy Environ. 7 (2022) 1093-1101.
Versatile control of concentration gradients in non-fullerene acceptor-based bulk heterojunction films using solvent rinse treatments
Chang-Mok Oh1, Soyeong Jang1, Jihoon Lee, Sung Heum Park*, In-Wook Hwang*
Material concentration gradient along the longitudinal direction of non-fullerene acceptor-based BHJ film, which is flexibly controlled by solvent rinse treatment using MeOH and n-hexane.
https://doi.org/10.1016/j.gee.2021.01.009
Citation: C.-M. Oh, S. Jang, J. Lee, S.H. Park, I.-W. Hwang, Green Energy Environ. 7 (2022) 1102-1110.
N-doped graphene anchored ultrasmall Ir nanoparticles as bifunctional electrocatalyst for overall water splitting
Wenqing Yao1, Xian Jiang1, Yulian Li, Cuiting Zhao, Linfei Ding, Dongmei Sun*, Yawen Tang*
The N-doped graphene anchored Ir nanoparticles (Ir/N-rGO) with ultrasmall particle size is synthesized via a simple hydrothermal method. Due to the synergy among ultrasmall Ir nanoparticle and N-doped rGO, the Ir/N-rGO exerts highly robust catalytic activity and durability toward the overall water splitting.
https://doi.org/10.1016/j.gee.2021.01.011
Citation: W. Yao, X. Jiang, Y. Li, C. Zhao, L. Ding, D. Sun, Y. Tang, Green Energy Environ. 7 (2022) 1111-1118.
Homodispersed B–CN/P–CN S-scheme homojunction for enhanced visible-light-driven hydrogen evolution
Dashui Yuan, Zongyuan Li, Xueru Chen, Jing Ding*, Hui Wan, Guofeng Guan*https://doi.org/10.1016/j.gee.2021.01.012
Citation: D. Yuan, Z. Li, X. Chen, J. Ding, H. Wan, G. Guan, Green Energy Environ. 7 (2022) 1119-1127.
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